• Wulff Thomson posted an update 6 months ago

    The increasing trends may be due to increased inputs from river discharges, the leather industry and petroleum refineries, while the decrease in Pb may be due to the ban in the use of this element as an additive in gasoline and as component of car batteries. This investigation supports the validity of analysing trace element in bone, a tissue available in scientific collections and museums, to retrospectively examine variation over long temporal scales and thus assess long-term trends in pollution.Coke resources are abundantly available worldwide and are a large by-product of tar production. Moreover, their utilization presents a series of environmental pollution problems. Common technologies for coal tar production applications urgently need to be upgraded because coal tar is listed as a national hazardous waste. This review associates coal tar development with deep processing technology for extracting environmentally beneficial compounds from coal tar, which have never been reported. Recent studies on the innovative approaches for extracting phenols and nitrogen-containing compounds from coal tar have been addressed, as well as a preparation method of carbon materials with high catalytic activity and a well-ordered structure by confined polymerization. Tremendous demand for further research and exploration of selectively extracted compounds from coal tar implies a new opportunity for polymerizing the resin and a great challenge for the current technology implemented for valorizing coal tar into ordered carbon materials. Consequently, more concerted efforts should be implemented to achieve a wide range of polymer resin applications and improve the quality of carbon precursors extracted from the coal tar, thus increasing the economic benefit and scientific value of coal tar.The co-existence of antibiotics and heavy metal (HM) is common in manure. However, existing strategies for improving antibiotic dissipation or HM immobilization during composting rarely consider their combined pollution. In this study, we used agricultural lime and a newly designed attapulgite-activated carbon composite (AACC) to enhance the stabilization of HMs in a pilot-scale swine manure composting system and assessed the effectiveness of these materials for removing antibiotic residues. Results indicated that the application of either lime or AACC simultaneously enhanced HM immobilization and antibiotic degradation. In particular, the addition of AACC reduced the enrichment of Cr, Cd, Pb, and As during composting and decreased the half-lives of the antibiotics from 10.7 days to 6.3 days, which were more effectively than lime. The physicochemical and microbiological responses to different additives were subsequently studied to understand the mechanisms underlying the fates of HMs and antibiotics. High HM stress in manure inhibited antibiotic dissipation, but metal immobilization alleviated this effect. The AACC accelerated HM immobilization by surface adsorption and metal precipitation, and this enhancement strengthened during the late composting stage due to an increase in pH, whereas lime exhibited a short-term effect. Moreover, the AACC addition enhanced the contribution of bacteria to changes in antibiotic concentrations, while the increase in pile temperature could be a major factor that contributed to the acceleration of antibiotic degradation after the addition of lime. Characterization of the final compost further showed that AACC-treated compost had the lowest residual concentrations of HMs and antibiotics, higher mortality of ascarid egg, improved nitrogen conversation, and reduced phytotoxicity. Thus, co-composting of swine manure with AACC is a promising approach for producing safer compost for use in agriculture.The planetary boundaries (PBs) delineating the safe operating space for human activities have been broadly recognized as a well-grounded framework for global sustainability assessment. This paper provides a comprehensive review of the application and methodological extensions of the PBs by linking with multiscale environmental sustainability assessments. We find that the targeted scales, sharing principles and sustainability perspectives jointly determine the downscaling of the PBs-a complex process that needs to take into account the biophysical, socioeconomic, ethical and cultural dimensions. Despite the varying sharing principles, in general both top-down and bottom-up approaches have been employed to define the environmental boundaries at sub-global scales on which the various PBs highly differ in their threshold behaviors. To clarify the responsibility of different stakeholders for sustainable development, the PB-informed sustainability assessment should refer to a specific perspective (i.e., production-, consumption-, or life cycle-based). Rapamycin Furthermore, the methodological extensions of PBs have the potential to monitor the progress and gaps of the globally consensus-based Sustainable Development Goals (SDGs). To achieve the SDGs within the PBs, there is a great need for a thorough transition of socioeconomic systems towards a prosperous, just and sustainable future.Although river restoration has been increasingly implemented to restore water quality in ecosystems, its effect on the removal of emerging pollutant antibiotics, and their resultant influence on microbial community structure and functions in river water is still unclear. This study investigated the changes of antibiotics, antibiotic resistant genes (ARGs), microbial communities, and their spatial distributions in a megacity river before and after river restoration. Results indicated that although the restoration activities including riverbed dredging, riverbank hardening, sewage and storm water separation and re-pipelining improved water quality such as by decreasing total phosphorus (TP) content from 4.60 ± 6.38 mg/L in 2018 to 0.98 ± 0.44 mg/L in 2020, the antibiotic concentrations in river water increased. Total antibiotic concentrations in the water samples were higher in 2020 (506.89-6952.50 ng/L) than those in 2018 (137.93-1751.51 ng/L), likely caused by increased usage of antibiotics in 2020 for COVID-19 treatment.

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